Doodles and jots has a really clever art project making paint brushes out of twigs and leaves, straw and grass. The great part is the fun continues after the brushes are made and they can see the different textures each brush makes.
Good for ages 7 and up.
Get the instructions here:
http://www.doodlesandjots.com/2012/01/05/making-paintbrushes-with-natural-materials/
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